H(+)-Assisted fluorescent differentiation of Cu(+) and Cu(2+): effect of Al(3+)-induced acidity on chemical sensing and generation of two novel and independent logic gating pathways.

نویسندگان

  • Yonghwang Ha
  • Dhiraj P Murale
  • Changsuk Yun
  • Sudesh T Manjare
  • Hyungjun Kim
  • Juhyoun Kwak
  • Yoon Sup Lee
  • David G Churchill
چکیده

A novel Schiff base probe exhibited strong 'turn-ON' fluorescence for Cu(2+) at 345 nm, Al(3+) at 445 nm, and Cu(+) at 360 nm in the presence of Al(3+) in organic solvent (acetonitrile), which allowed for construction of molecular logic gates 'INH' and '1:2 DEMULTIPLEXING.' H(+) generated from Al(3+) contributed greatly to Cu(+) chemosensing based on a redox non-innocence mechanism.

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عنوان ژورنال:
  • Chemical communications

دوره 51 29  شماره 

صفحات  -

تاریخ انتشار 2015